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CO2的还原转化反应研究 Title:CO2ReductionandConversionReactions:AComprehensiveStudy Abstract: Thereductionandconversionofcarbondioxide(CO2)havegarneredsignificantattentioninrecentyearsduetotheurgentneedforsustainableenergyproductionandenvironmentalprotection.Thispaperaimstoprovideacomprehensivereviewofthevariousreactionpathways,catalysts,andexperimentalapproachesemployedinthestudyofCO2reductionandconversion.Furthermore,thepotentialapplicationsofthesereactionsintheproductionofvalue-addedproductsandtheirimpactonmitigatingCO2emissionsarediscussed.ThefindingshighlighttheimportanceofcontinuedresearchinthisfieldtoestablisheconomicallyviableandenvironmentallyfriendlysolutionsforCO2utilization. 1.Introduction 1.1BackgroundandMotivation 1.2ObjectivesandScope 1.3Methodology 2.CO2ReductionMechanisms 2.1ElectrochemicalReduction 2.1.1Fundamentals 2.1.2CatalystsandElectrocatalyticProcesses 2.2PhotocatalyticReduction 2.2.1Mechanisms 2.2.2SemiconductorPhotocatalysts 2.2.3PhotocatalyticSystems 2.3BiologicalCO2Conversion 2.3.1MicrobialConversion 2.3.2EnzymaticConversion 3.CatalystsforCO2Reduction 3.1MetalCatalysts 3.2Metal-FreeCatalysts 3.3HybridCatalysts 3.4EmergingCatalysts 4.ExperimentalApproachesandTechniques 4.1ElectrochemicalTechniques 4.1.1CyclicVoltammetry 4.1.2Chronoamperometry 4.1.3ElectrochemicalImpedanceSpectroscopy 4.2SpectroscopicTechniques 4.2.1FourierTransformInfraredSpectroscopy 4.2.2Ultraviolet-VisibleSpectroscopy 4.2.3X-rayPhotoelectronSpectroscopy 4.3CharacterizationTechniques 4.3.1ScanningElectronMicroscopy 4.3.2TransmissionElectronMicroscopy 4.3.3X-rayDiffraction 5.ApplicationsandChallenges 5.1FuelGeneration 5.2ChemicalFeedstockProduction 5.3EnvironmentalApplications 5.4EconomicandEnvironmentalConsiderations 5.5ChallengesandFuturePerspectives 6.Conclusion 6.1SummaryofKeyFindings 6.2RecommendationsforFutureResearch ThecomprehensivestudypresentedinthispaperhighlightsthepromisingpotentialofCO2reductionandconversionreactionsasaneffectivestrategyinmitigatingCO2emissionsandprod